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Enhancing the electricity generation and sludge reduction of sludge microbial fuel cell with graphene oxide and reduced graphene oxide

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Indexed by:期刊论文

First Author:Zhang, Hanmin

Correspondence Author:Zhang, HM (reprint author), Linggong Rd 2, Dalian 116024, Peoples R China.; Feng, YJ (reprint author), 73 Huanghe Rd, Harbin 150090, Heilongjiang, Peoples R China.

Co-author:Da, Zongyang,Feng, Yujie,Wang, Yuezhu,Cai, Lu,Cui, Hongtao

Date of Publication:2018-06-10

Journal:JOURNAL OF CLEANER PRODUCTION

Included Journals:SCIE、EI

Volume:186

Page Number:104-112

ISSN No.:0959-6526

Key Words:Sludge microbial fuel cell; Graphene oxide; Reduced graphene oxide; Sludge reduction; Electricity production

Abstract:Sludge microbial fuel cell (SMFC) is capable of extracting biomass energy directly from the sludge while generating electricity. However, most of organic matters in the excess sludge are the cell substances that are difficult to be used by microorganism directly. In this paper, adding graphene oxide (GO) and reduced graphene oxide (rGO) in SMFC was proposed and their advantages were reflected by no requiring external energy, in-situ promoting the electricity production and reducing sludge effectively. The results showed that the contents of lactate dehydrogenase (LDH) for adding 0.4 g GO in SMFC (0.4-GO SMFC) and adding 0.4 g rGO in SMFC (0.4-rGO SMFC) were 2 and 1.81 times higher than that of adding nothing in SMFC (ordinary SMFC), respectively. The species and compositions of organic matter in 0.4-GO SMFC and 0.4-rGO SMFC decreased significantly and their sludge reduction rate were 3 and 2.2 times that of ordinary SMFC, respectively. Comparing with ordinary SMFC, the maximum power density of 0.4-GO SMFC and 0.4-rGO SMFC was up to 214.09 and 80.52 mW m(-3) separately, and their internal resistance decreased by 71% and 48%, respectively. Thus, it can be concluded that GO and rGO had the function of breaking cell and accelerated electrons transporting, so they could greatly promote the sludge reduction and electricity production of SMFC. (C) 2018 Published by Elsevier Ltd.

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