张捍民

个人信息Personal Information

教授

博士生导师

硕士生导师

性别:女

毕业院校:哈尔滨工业大学

学位:博士

所在单位:环境学院

学科:环境工程. 环境科学

电子邮箱:zhanghm@dlut.edu.cn

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Operation adjustments of an electrochemically coupled system for total nitrogen removal and the associated mechanism

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论文类型:期刊论文

发表时间:2020-05-01

发表刊物:Chemosphere

收录刊物:EI、PubMed

卷号:246

页面范围:125649

ISSN号:1879-1298

关键字:Electrochemical denitrification,Microbial fuel cell,Phosphorus accumulating organisms,Polyhydroxyalkanoate,Sequencing batch reactor

摘要:A coupled system consisting of sequencing batch reactor and microbial fuel cell (SBR-MFC) was designed to buffer pH drift and purify wastewater. The addition of nitrifying sludge and the adjustment of hydraulic retention time (HRT) were performed to achieve better removal of total nitrogen (TN). When anaerobic/aerobic/anoxic phases in one cycle were 6/4/2 h, the removal efficiency of ammonium was 99.0 ± 1.3%, whereas denitrification was insufficient and the overall removal efficiency of TN was only 29.1 ± 5.8%. When the phases were adjusted to 6/2/4 h, the removal efficiencies of ammonium were 100.0 ± 0.0% in both closed and open circuits, and the overall removal efficiencies of TN were 91.4 ± 0.2% and 71.7 ± 4.2%, respectively, improved by 20% in MFC mode; the maximum voltage (200 Ω) maintained at 0.1 V. Ammonium-oxidizing bacteria (AOB) and Nitrite-oxidizing bacteria (NOB) in the sludge carried out nitrification. The main denitrification pathways in anoxic phase involved polyhydroxyalkanoate (PHA) denitrification by denitrifying glycogen accumulating organisms (GAOs) and electrochemical denitrification by electrochemical active bacteria (EAB). Few polyphosphate accumulating organisms (PAOs) were present, which accounted for poor P removal.Copyright © 2019 Elsevier Ltd. All rights reserved.