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论文类型：期刊论文

发表时间：2021-03-05

发表刊物：PHYSICAL REVIEW A

卷号：102

期号：6

ISSN号：2469-9926

摘要：Field-free molecular orientation, achieved by using two-color slow turn-on and rapid turn-off laser pulses, is theoretically investigated for linear molecules. We derive analytical results for the maximum degree of field-free orientation for a given number of populated rotational states. We show that numerical results with adiabatic-turnon and sudden-turn-off laser pulses attain the optimal orientation. Based on the adiabatic theorem, the effects of laser and molecular parameters on both the adiabatic process and the degree of molecular orientation are analyzed. The adiabaticity is well reflected through the temporal evolution of the phase difference between two adjacent rotational states.