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    • 教授     博士生导师   硕士生导师
    • 性别:男
    • 毕业院校:奥地利University of Graz
    • 学位:博士
    • 所在单位:环境学院
    • 学科:环境工程. 环境科学. 水科学与技术
    • 办公地点:大连理工大学环境学院
    • 联系方式:0411-84706140
    • 电子邮箱:quanxie@dlut.edu.cn

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    Three-dimensional TiO2 nanotube arrays combined with g-C3N4 quantum dots for visible light-driven photocatalytic hydrogen production

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    论文类型:期刊论文

    发表时间:2017-01-01

    发表刊物:RSC ADVANCES

    收录刊物:SCIE、EI

    卷号:7

    期号:22

    页面范围:13223-13227

    ISSN号:2046-2069

    摘要:A three-dimensional (3D) nanostructured photocatalyst combined with g-C3N4 quantum dots (QDs) and a TiO2 nanotube array (TNA) was fabricated to form a 3D g-C3N4/ TNA nanocomposite by a facile electro-deposition process. The photocatalytic ability of the 3D g-C3N4/ TNA was evaluated by measuring the amount of hydrogen generated from water splitting under visible light irradiation. Benefiting from an attractive heterostructure between g-C3N4 and TiO2 leading to a unique photogenerated charge separation, as well as a distinctive 3D well-ordered nanotube structure, this 3D g-C3N4/ TNA exhibited an average H-2 production of approximately 243 mmol h(-1) g(-1), which was approximately 4.7 times higher than that of sole g-C3N4 under the same experimental conditions. Therefore, this work could offer a prospective 3D nanostructure for visible light-driven photocatalytic applications.