个人信息Personal Information
教授
博士生导师
硕士生导师
性别:男
毕业院校:大连理工大学
学位:博士
所在单位:电气工程学院
学科:环境工程. 电工理论与新技术. 高电压与绝缘技术
办公地点:大连理工大学电气工程学院静电所
Effects of electrode geometry on the performance of dielectric barrier/packed-bed discharge plasmas in benzene degradation
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论文类型:期刊论文
发表时间:2013-11-15
发表刊物:JOURNAL OF HAZARDOUS MATERIALS
收录刊物:SCIE、EI、PubMed、Scopus
卷号:262
页面范围:387-393
ISSN号:0304-3894
关键字:Benzene; Electrode geometry; Dielectric barrier discharge; Packed-bed discharge
摘要:In this study, the effects of electrode geometry on benzene degradation in a dielectric barrier/packed-bed discharge plasma reactor with different electrodes were systematically investigated. Three electrodes were employed in the experiments, these were coil, bolt, and rod geometries. The reactor using the coil electrode showed better performance in reducing the dielectric loss in the barrier compared to that using the bolt or rod electrodes. In the case of the coil electrode, both the benzene degradation efficiency and energy yield were higher than those for the other electrodes, which can be attributed to the increased role of surface mediated reactions. Irrespective of the electrode geometry, the packed-bed discharge plasma was superior to the dielectric barrier discharge plasma in benzene degradation at any specific applied voltage. The main gaseous products of benzene degradation were CO, CO2, H2O, and formic acid. Discharge products such as O-3, N2O, N2O5, and HNO3 were also detected in the outlet gas. Moreover, the presence of benzene inhibited the formation of ozone because of the competing reaction of oxygen atoms with benzene. This study is expected to offer an optimized approach combining dielectric barrier discharge and packed-bed discharge to improve the degradation of gaseous pollutants. (C) 2013 Elsevier B.V. All rights reserved.