点击次数：

论文类型：期刊论文

发表时间：2018-02-01

发表刊物：FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING

收录刊物：SCIE、Scopus

卷号：12

期号：1

ISSN号：2095-2201

关键字：Reduced graphene oxide; Au; TiO2; Nanocomposite; Photocatalysis

摘要：A new type of Au/TiO2/reduced graphene oxide (RGO) nanocomposite was fabricated by the hydrothermal synthesis of TiO2 on graphene oxide followed by the photodeposition of Au nanoparticles. Transmission electron microscopy images showed that Au nanoparticles were loaded onto the surface of both TiO2 and RGO. Au/TiO2/RGO had a better photocatalytic activity than Au/TiO2 for the degradation of phenol. Electrochemical measurements indicated that Au/TiO2/RGO had an improved charge transfer capability. Meanwhile, chemiluminescent analysis and electron spin resonance spectroscopy revealed that Au/TiO2/RGO displayed high production of hydrogen peroxide and hydroxyl radicals in the photocatalytic process. This high photocatalytic performance was achieved via the addition of RGO in Au/TiO2/RGO, where RGO served not only as a catalyst support to provide more sites for the deposition of Au nanoparticles but also as a collector to accept electrons from TiO2 to effectively reduce photogenerated charge recombination. (C) Higher Education Press and Springer-Verlag Berlin Heidelberg 2017