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Rhodium-Catalyzed Oxidative Benzannulation of N-Adamantyl-1-naphthylamines with Internal Alkynes via Dual C-H Bond Activation: Synthesis of Substituted Anthracenes

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期刊论文
First Author:
Zhang, Xuan
Correspondence Author:
Yu, XQ; Bao, M (reprint author), Dalian Univ Technol, State Key Lab Fine Chem, Dalian 116023, Peoples R China.
Co-author:
Yu, Xiaoqiang,Ji, Dingwei,Yamamoto, Yoshinori,Almansour, Abdulrahman I.,Arumugam, Natarajan,Kumar, Raju Suresh,Bao, Ming
Date of Publication:
2016-09-02
Journal:
ORGANIC LETTERS
Included Journals:
SCIE、PubMed、Scopus
Document Type:
J
Volume:
18
Issue:
17
Page Number:
4246-4249
ISSN No.:
1523-7060
Abstract:
Rhodium-catalyzed oxidative benzannulation of N-adaffianty1-1-naphthylarnines with internal alkynes to produce highly substituted anthracenes in satisfactory to good yields was developed. The annulation reaction proceeded smoothly under mild conditions in the presence of [Cp*RhCl2](2) as the precatalyst and Cu(OAc)(2) as the oxidant.

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