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个人信息Personal Information
教授
博士生导师
硕士生导师
主要任职：Professor Dr. Hongbin Ding
其他任职：物理学院学术委员会主任，等离子体联合研究中心主任,中国光学工程学会LIBS专委会副主任, 中国核学会核聚变等离子体分会常务理事，辽宁省物理学会副理事长，国际ITER-ITPA 委员
性别：男
毕业院校：巴塞尔大学
学位：博士
所在单位：物理学院
学科：等离子体物理. 光学工程
联系方式：hding@dlut.edu.cn
电子邮箱：hding@dlut.edu.cn
High-Sensitivity In-Situ Diagnosis of NO2 Production and Removal in DBD Using Cavity Ring-Down Spectroscopy
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论文类型：期刊论文
发表时间：2014-02-01
发表刊物：PLASMA SCIENCE & TECHNOLOGY
收录刊物：SCIE、EI、Scopus
卷号：16
期号：2
页面范围：142-148
ISSN号：1009-0630
关键字：DBD; CRDS; NO2 production; NO2 removal
摘要：A highly-sensitive in-situ diagnosis approach for nitrogen dioxide (NO2) has been developed in dielectric barrier discharge (DBD) based on pulsed cavity ring-down spectroscopy (CRDS). Absorption bands of NO2 in a spectral region from 508 nm to 509 nm were used, and a detection limit of 17.5 ppb was achieved. At this level of sensitivity, the quantitative and real-time monitoring of the production and removal of NO2 are accomplished for the first time in the discharge region. By measuring the removal amount and rate at different NO2 initial number densities from 1.54 x 10(13) cm(-3) to 2.79 x 10(14) cm(-3), we determined the relationship between them and NO2 initial number densities. The removal amount linearly increases with the initial number density, while the removal rate increases logarithmically. At a lower initial number density, the removal rate is limited. By considering the chemical kinetic mechanism in plasma, a qualitative explanation for the above phenomena is proposed: the additional NO2 produced by discharge limits the removal rate, since the NO2 concentration is dominated by the competition between the forward reactions (production) and the reverse reactions (removal).