宋学志

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副教授

博士生导师

硕士生导师

性别:男

毕业院校:中国科学院大学

学位:博士

所在单位:化工海洋与生命学院

办公地点:D03-302

联系方式:15604270228

电子邮箱:songxz@dlut.edu.cn

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Metal-organic framework-derived porous CeO2 loading Au as efficient nanocatalysts for CO oxidation and 4-nitrophenol reduction

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论文类型:期刊论文

发表时间:2018-06-01

发表刊物:FUNCTIONAL MATERIALS LETTERS

收录刊物:SCIE

卷号:11

期号:3

ISSN号:1793-6047

关键字:Au/CeO2; CO oxidation; 4-nitrophenol reduction; metal-organic frameworks

摘要:In this paper, two Au/CeO2 catalytic systems have been fabricated through the synthesis of porous CeO2 from Ce-BTC MOFs nanorod and nanobundle precursors by thermal annealing, and the subsequent Au loading. Significantly, the catalytic activity of Au/CeO2 nanorods is higher than that of bare CeO2 and even Au/CeO2 nanobundles for both CO oxidation and 4-nitrophenol reduction. The remarkably enhanced performance of Au/CeO2 nanorods can be attributed to the unique porous structure, high surface area, abundant oxygen vacancies on the surface of CeO2, and the synergistic effect between gold and ceria.