李新勇

个人信息Personal Information

教授

博士生导师

硕士生导师

性别:男

毕业院校:中国科学院兰州化学物理研究所

学位:博士

所在单位:环境学院

办公地点:环境楼 B415

联系方式:Tel: 0411-84706658

电子邮箱:xyli@dlut.edu.cn

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Multifunctional Plasmonic Co-Doped Fe2O3@polydopamine-Au for Adsorption, Photocatalysis, and SERS-based Sensing

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论文类型:期刊论文

发表时间:2016-09-01

发表刊物:PARTICLE & PARTICLE SYSTEMS CHARACTERIZATION

收录刊物:SCIE、EI、Scopus

卷号:33

期号:9

页面范围:602-609

ISSN号:0934-0866

关键字:composite materials; photocatalysis; SERS sensors; surface plasmon resonance

摘要:A new type of multifunctional plasmonic nanoparticles, cobalt-doped Fe2O3@polydopamine-Au (Co-Fe2O3@PDA-Au), is fabricated via coating PDA through self-polymerization onto Co-Fe2O3 and further loading gold nanoparticles by in situ reduction onto the surface of PDA shell. Benefiting from the universal adhesive ability of PDA and negative zeta potetntial of the composite, the Co-Fe2O3@PDA-Au shows strong adsorptivity for cationic dyes. The presence of gold nanoparticle with the diameter of 15 nm in the Co-Fe2O3@PDA-Au system promotes surface-enhanced Raman scattering (SERS) activity with an impressive detection limit of 1 x 10(-6) m. Thanks to the synergistic effect of the light harvesting of PDA, the surface plasmon resonance of Au, and the electron conductibility of PDA and Au, the Co-Fe2O3@PDA-Au exhibits an enhanced photocatalytic activity comparing with unmodified Co-Fe2O3. All the above-mentioned functions enable Co-Fe2O3@PDA-Au to be a multifunctional material system for various applications toward environmental pollutants.