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个人信息Personal Information
教授
博士生导师
硕士生导师
性别：男
毕业院校：中国科学院兰州化学物理研究所
学位：博士
所在单位：环境学院
办公地点：环境楼 B415
联系方式：Tel: 0411-84706658
电子邮箱：xyli@dlut.edu.cn
Sulfur vacancy-rich N-doped MoS2 nanoflowers for highly boosting electrocatalytic N-2 fixation to NH3 under ambient conditions
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论文类型：期刊论文
发表时间：2019-06-28
发表刊物：CHEMICAL COMMUNICATIONS
收录刊物：SCIE
卷号：55
期号：51
页面范围：7386-7389
ISSN号：1359-7345
摘要：In this communication, optimized sulfur vacancy-rich nitrogen-doped MoS2 nanoflowers were developed, which served as excellent N-2 reduction reaction (NRR) electrocatalysts for the conversion of N-2 to NH3 under ambient conditions. Electrochemical results demonstrated that the as-prepared N-doped MoS2 electrode afforded a superior NH3 yield and high faradaic efficiency, which exceeded those of the recently reported MoS2 catalysts. The possible NRR catalytic mechanism and electron transfer pathway were further elucidated via density functional theory calculations.