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论文类型：期刊论文

发表时间：2016-06-01

发表刊物：GREENHOUSE GASES-SCIENCE AND TECHNOLOGY

收录刊物：SCIE、EI、Scopus

卷号：6

期号：3

页面范围：401-415

ISSN号：2152-3878

关键字：CO2 storage; heterogeneity; porous media; wettability; X-ray CT

摘要：The geological sequestration of carbon dioxide (CO2) is considered a promising technology for CO2 emissions. However, accurate estimation of the storage capacity for CO2 remains a challenge owing to the effect of capillary pressure variation. The CO2-salty aqueous contact angle and sub-core scale heterogeneity are the major factors that influence capillary pressure. This paper reports the results of CO2/brine two-phase flow experiments in porous media by using an X-ray computed tomography (CT) technique at 40 degrees C and 8 Mpa and examines the strong influence of wettability and sub-core scale heterogeneities on the spatial distribution of CO2. Gas injection experiments were conducted at flow rates of 0.1 mL/min, 0.2 mL/min, and 0.5 mL/min, and the porous media were packed with feldspar, quartz, or dolomite. This study indicates that at the core scale, the wettability of porous media is a crucial factor in determining CO2 saturation. Capillary fingering and low CO2 saturation occurred with high water wettability. Sub-core scale heterogeneities controlled the CO2 distribution and saturation variation along the porous media, particular that with small pore sizes. (c) 2015 Society of Chemical Industry and John Wiley & Sons, Ltd