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个人信息Personal Information
教授
博士生导师
硕士生导师
主要任职:无
其他任职:精细化工国家重点实验室副主任、大连理工大学-瑞典皇家工学院分子器件联合研究中心主任
性别:男
毕业院校:大连理工大学
学位:博士
所在单位:化工学院
学科:应用化学. 精细化工
办公地点:大连理工大学西部校区化工实验楼E-223
联系方式:0411-84986493
电子邮箱:sunlc@dlut.edu.cn
Simple Nickel-Based Catalyst Systems Combined With Graphitic Carbon Nitride for Stable Photocatalytic Hydrogen Production in Water
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论文类型:期刊论文
发表时间:2012-11-01
发表刊物:CHEMSUSCHEM
收录刊物:SCIE、EI、PubMed、Scopus
卷号:5
期号:11
页面范围:2133-2138
ISSN号:1864-5631
关键字:carbon nitrides; hydrogen production; nickel; photocatalysis; water splitting
摘要:A molecular catalyst system containing only earth-abundant elements is combined with g-C3N4 as photosensitizer. The in situ generated complexes serve as catalysts for visible-light-driven H2 production in aqueous solution, and do not require organic solvent or a Brønsted acid. H2 evolution from the Ni-based catalyst system can be maintained for over 60 h, demonstrating that the combination is a promising approach to improve the lifetimes of molecular catalysts towards photochemical H2 production. © 2012 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.