个人信息Personal Information
教授
博士生导师
硕士生导师
性别:男
毕业院校:中国科学院大连化学物理研究所
学位:博士
所在单位:环境学院
学科:环境科学. 环境工程
办公地点:大连理工大学西部校区环境楼B623
联系方式:tanf@dlut.edu.cn
Preparation of polydopamine-coated graphene oxide/Fe3O4 imprinted nanoparticles for selective removal of fluoroquinolone antibiotics in water
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论文类型:期刊论文
发表时间:2017-07-18
发表刊物:SCIENTIFIC REPORTS
收录刊物:SCIE、PubMed
卷号:7
期号:1
页面范围:5735
ISSN号:2045-2322
摘要:Antibiotics in water have recently caused increasing concerns for public health and ecological environments. In this work, we demonstrated polydopamine-coated graphene oxide/Fe3O4 (PDA@ GO/Fe3O4) imprinted nanoparticles coupled with magnetic separation for fast and selective removal of fluoroquinolone antibiotics in water. The nanoparticles were prepared by the self-polymerization of dopamine using sarafloxacin as a template. The imprinted PDA film of 10 similar to 20 nm uniformly covered the surface of GO/Fe3O4 providing selective binding sites. The nanoparticles showed rapid binding and a large capacity (70.9 mg/g). The adsorption data fitted well the Langmuir and pseudo-second order kinetic equations. The nanoparticles could be easily separated by a magnet following the adsorption and then regenerated by simple washing for repetitive adsorptions. The nanoparticles were successfully used for the removal of fluoroquinolone antibiotics in seawater, with removal efficiencies of more than 95%. The proposed strategy has potentials for efficient removal of antibiotics in environmental water.