个人信息Personal Information
副教授
博士生导师
硕士生导师
性别:男
毕业院校:武汉大学
学位:博士
所在单位:化工学院
电子邮箱:gzhang@dlut.edu.cn
个人简介Personal Profile
张光辉,博士,副教授,博士生导师,目前担任Journal of Energy Chemistry、Transactions of Tianjin University、Carbon Neutrality、《低碳化学与化工》等期刊青年编委。2007年毕业于南京师范大学化学专业获学士学位;2010年毕业于南京师范大学有机化学专业孙培培教授课题组获硕士学位;2014年毕业于武汉大学有机化学专业雷爱文教授课题组获得博士学位,攻读博士学位期间曾于2012年-2014年在美国阿贡国家实验室合作研究。获得博士学位之后,曾先后在美国伊利诺伊理工学院化学系/阿贡国家实验室Adam S. Hock教授课题组、普渡大学化工学院Jeffrey T. Miller教授课题组任博士后研究员,并于2018年加入大连理工大学化工学院郭新闻教授团队。目前研究兴趣集中在多相催化领域,利用动态、原位光谱学方法研究二氧化碳、烷烃等小分子催化转化反应中表界面活性位、反应物种和表面动态结构。入选“兴辽英才计划”青年拔尖人才、大连市青年才俊、大连理工大学“星海青千”、化工学院“大煜学者”优秀青年人才等,曾获得Molecular Catalysis Young Researcher Award、Energy & Fuels Rising Stars、Industrial & Engineering Chemistry Research Influential Researcher等奖励和荣誉,承担国家自然科学基金面上项目、青年基金、新疆维吾尔自治区重大科技专项子课题等科研项目多项。发表SCI论文100余篇,据Web of Science统计,论文被引7000余次,H因子为49,获授权中国发明专利1件,美国发明专利3件。
欢迎具有化学、化工、材料背景,对纳米材料、多相催化、催化剂原位表征、二氧化碳与烷烃等小分子催化转化感兴趣的同学加入我们研究团队(郭新闻教授领衔“兴辽英才计划”高水平创新创业团队、辽宁省优秀研究生导师团队)。
博士后招聘专业:化学工程与技术
博士生招生专业:化学工程与技术(工业催化)学术型博士(学制4年)
硕士生招生专业:化学工程与技术(工业催化)学术型硕士(学制3年)、化学工程专业硕士(限催化化工方向,学制3年)
联系方式:gzhang@dlut.edu.cn
主持科研项目
1)碳化物界面催化剂原位制备及其在二氧化碳加氢反应中的应用研究,国家自然科学基金面上项目
2)二氧化碳加氢反应中复合金属氧化物催化剂表面重构探究,国家自然科学基金面上项目
3)铂基双金属纳米催化剂用于二氧化碳氧化丙烷脱氢反应研究,国家自然科学基金青年基金
4)二氧化碳催化转化新材料与结构演变机制,兴辽英才计划青年拔尖人才项目
5)燃煤烟气多污染物联合脱除及CO2捕集利用技术研究,新疆维吾尔自治区重大科技专项子课题
6)二氧化碳转化中钴基催化剂定向调控,中央高校基本科研业务费理科基础科研专题
7)锌基催化剂用于二氧化碳催化转化研究,中央高校基本科研业务费引进人才专项
8)烷烃及二氧化碳催化转化研究,中央高校基本科研业务费引进人才专项
Selected Publications Since 2018
Research papers
1) Wu, Z.; Bukowski, B. C.; Li, Z.; Milligan, C.; Zhou, L.; Ma, T.; Wu, Y.; Ren, Y.; Ribeiro, F. H.; Delgass, W. N.; Greeley, J.; Zhang, G.*; Miller, J. T.*: Changes in Catalytic and Adsorptive Properties of 2 nm Pt3Mn Nanoparticles by Subsurface Atoms. J. Am. Chem. Soc. 2018, 140, 14870-14877
2) Cesar, L.G.; Yang, C.; Lu, Z.; Ren, Y.; Zhang, G.*; Miller, J.T.*: Identification of a Pt3Co Surface Intermetallic Alloy in Pt-Co Propane Dehydrogenation Catalysts. ACS Catal. 2019, 9, 5231-5244
3) Zhang, G.#; Ye, C.#; Liu, W.; Zhang, X.; Su, D.; Yang, X.; Zhu Chen, J.; Wu, Z.*; Miller, J. T.*: Diffusion Limited Formation of Non-Equilibrium Intermetallic Nanophase for Selective Dehydrogenation. Nano Lett. 2019, 19, 4380-4383
4) Wang, J.#; Liu, C.-Y.#; Senftle, T.P.; Zhu, J.; Zhang, G.*; Guo, X.*; Song, C.*: Variation in the In2O3 Crystal Phase Alters Catalytic Performance toward the Reverse Water Gas Shift Reaction. ACS Catal. 2020, 10, 3264-3273 (cover)
5) Zhu, J.; Zhang, G.*; Li, W.; Zhang, X.; Ding, F.; Song, C.*; Guo, X.*: Deconvolution of the Particle Size Effect on CO2 Hydrogenation over Iron-based Catalysts. ACS Catal. 2020, 10, 7424-7433
6) Wan, G.; Zhang, G.*; Lin, X.-M.*: Toward Efficient Carbon and Water Cycles: Emerging Opportunities with Single-Site Catalysts Made of 3d Transition Metals. Adv. Mater. 2020, 32, 1905548
7) LiBretto, N.#; Xu, Y.#; Quigley, A.; Edwards, E.; Nargund, R.; Vega-Vila, J.; Saxena, A.; Gounder, R.; Greeley, J.; Zhang, G.*; Miller, J.T.*: Olefin Oligomerization by Main Group Ga3+ and Zn2+ Single Site Catalysts on SiO2. Nat. Commun. 2021, 12, 2322
8) Wang, J.; Zhang, G.*; Zhu, J.; Zhang, X.; Ding, F.; Zhang, A.; Guo, X.*; Song, C.*: CO2 Hydrogenation to Methanol over In2O3-based Catalysts: From Mechanism to Catalyst Development. ACS Catal. 2021, 11, 1406-1423 (ESI Highly Cited Paper)
9) Zhang, X.; Zhang, G.*; Liu, W.; Yuan, F.; Wang, J.; Zhu, J.; Jiang, X.; Zhang, A.; Ding, F.; Song, C.*; Guo, X.*: Reaction-Driven Surface Reconstruction of ZnAl2O4 Boosts the Methanol Selectivity in CO2 Catalytic Hydrogenation. Appl. Catal. B: Environ. 2021, 284, 119700
10) Liu Y.; Zhang, G.*; Wang, J.; Zhu, J.; Zhang, X.; Miller, J.T.; Song, C.*; Guo, X.*: Promoting Propane Dehydrogenation with CO2 over Ga2O3/SiO2 by Eliminating Ga-Hydrides. Chin. J. Catal. 2021, 42, 2225-2233
11) Zhu, J.; Wang, P.; Zhang, X.; Zhang, G.*; Li, R.; Li, W.; Senftle, T.P.; Liu, W.; Wang, J.; Wang, Y.; Zhang, A.; Fu, Q.; Song, C.*; Guo, X.*: Dynamic Structural Evolution of Iron Catalysts Involving Competitive Oxidation and Carburization during CO2 Hydrogenation. Sci. Adv. 2022, 8, eabm3629 (ESI Highly Cited Paper)
12) Wang, M.; Zhang, G.*; Zhu, J.; Li, W.; Wang, J.; Bian, K.; Liu, Y.; Ding, F.; Song, C.*; Guo, X.*: Unraveling the Tunable Selectivity on Cobalt Oxide and Metallic Cobalt Sites for CO2 Hydrogenation. Chem. Eng. J. 2022, 446, 137217
13) Bian, K.; Zhang, G.*; Zhu, J.; Wang, X.; Wang, M.; Lou, F.; Liu, Y.; Song, C.*; Guo,X.*: Promoting Propane Dehydrogenation with CO2 over PtFe Bimetallic Catalyst by Eliminating the Non-selective Fe(0) Phase. ACS Catal. 2022,12, 6559-6569
14) Wan, G.*; Zhang, G.*; Zhu Chen, J.; Toney, M. F.*; Miller, J. T.*; Tassone, C. J.*: Reaction-mediated Transformation of Working Catalysts. ACS Catal. 2022, 12, 8007-8018
15) Liu, Y.; Zhang, G.*; Liu, S.; Zhu, J.; Liu, J.; Wang, J.; Li, R.; Wang, M.; Fu, Q.; Hou, S.*; Song, C.*; Guo, X.*: Promoting n-Butane Dehydrogenation over PtMn/SiO2 through Structural Evolution Induced by a Reverse Water-Gas Shift Reaction. ACS Catal. 2022, 12, 13506–13512
16) Wang, M.; Wang, P.; Zhang, G.*; Cheng, Z.; Zhang, M.; Liu, Y.; Li, R.; Zhu, J.; Wang, J.; Bian, K.; Liu, Y.; Ding, F.; Senftle, T.P.*; Nie, X.; Fu, Q.; Song, C.*; Guo, X.*: Stabilizing Co2C with H2O and K promoter for CO2 hydrogenation to C2+ hydrocarbons. Sci. Adv. 2023, 9, eadg0167
17) Wang, H.; Yang, C.; Yu, X.; Wang, M.; Yang, R.; Nie, X.; Yin, B.H.; Yip, A.C.K.; Song, C.; Zhang, G.*; Guo, X.*: Triple the Steady-State Reaction Rate by Decorating the In2O3 Surface with SiOx for CO2 Hydrogenation. J. Energy Chem., 2024, 95, 96-105
18) Wang, M.; Zhang, G.*; Wang, H.; Wang, Z.; Zhou, Y.; Nie, X.; Yin, B.H.; Song, C.*; Guo, X.*: Understanding and Tuning the Effects of H2O on Catalytic CO and CO2 Hydrogenation. Chem. Rev. 2024, 124, 12006-12085
19) Zhang, M.; Zhang, L.; Wang, M.; Zhang, G.*; Song, C.; Guo, X.*: The Electronic Interaction of Encapsulating Graphene Layers with FeCo Alloy Promotes Efficient CO2 Hydrogenation to Light Olefins. Chin. J. Catal. 2024, accepted
20) Liu, N.; Fan, Q.; Wei, J.*; Zhang, G.*; Sun, J.; Li, W.; Song, C.; Guo, X.*: Fine-tuning the active phases of CoFe alloy carbides for boosting olefin synthesis from CO2 hydrogenation. ACS Catal. 2024, accepted
A full list of publications could be found at ORCID and Web of Science.
https://orcid.org/0000-0002-5854-6909
https://www.webofscience.com/wos/author/record/1395849
Book Chapters
1) Zhang, G.; LiBretto, N.; Purdy, S.; Cesar, L.; Miller, J: (2023). X-Ray Absorption Spectroscopy (XAS): Surface Structural Determination of Alloy Nanoparticles. In: Wachs, I.E., Bañares, M.A. (eds) Springer Handbook of Advanced Catalyst Characterization. Springer Handbooks. Springer, Cham. https://doi.org/10.1007/978-3-031-07125-6_30
Patents
1) 郭新闻,刘军辉,张光辉,宋春山:CO2加氢制烃含碳铁基催化剂及其制备方法, 专利号:201910714776.2,授权日期2021年11月23日
2) Miller, J. T.; Zhang, G.: Phosphate-promoted Nickel Catalyst for High Temperature Oligomerization. US Patent, (美国专利号:US11135573B2; 授权日期:2021年10月5日).
3) Krause, T. R.; Hock, A. S.; Zhang, G.; Xu, Y.: Alkane Activation with Single and Bi-metallic Catalysts. US patent (美国专利号:US11034627B2; 授权日期:2021年6月15日).
4) Krause, T. R.; Hock, A. S.; Zhang, G.; Xu, Y.: Alkane Activation with Single and Bi-metallic Catalysts. US patent (美国专利号:US10472303B2; 授权日期:2019年11月12日).