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论文类型：期刊论文

发表时间：2016-10-01

发表刊物：CHINESE PHYSICS B

收录刊物：SCIE、EI、ISTIC、Scopus

卷号：25

期号：10

ISSN号：1674-1056

关键字：atmospheric-pressure plasma jet; hydrocarbon; OH radicals; laser-induced fluorescence

摘要：In this paper, a pulsed-dc CH3OH/Ar plasma jet generated at atmospheric pressure is studied by laser-induced fluorescence (LIF) and optical emission spectroscopy (OES). A gas-liquid bubbler system is proposed to introduce the methanol vapor into the argon gas, and the CH3OH/Ar volume ratio is kept constant at about 0.1%. Discharge occurs in a 6-mm needle-to-ring gap in an atmospheric-pressure CH3OH/Ar mixture. The space-resolved distributions of OH LIF inside and outside the nozzle exhibit distinctly different behaviors. And, different production mechanisms of OH radicals in the needle-to-ring discharge gap and afterglow of plasma jet are discussed. Besides, the optical emission lines of carbonaceous species, such as CH, CN, and C-2 radicals, are identified in the CH3OH/Ar plasma jet. Finally, the influences of operating parameters (applied voltage magnitude, pulse frequency, pulsewidth) on the OH radical density are also presented and analyzed.