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个人信息Personal Information
教授
博士生导师
硕士生导师
任职 : 现任大连理工大学化工学院教授、博士生导师。同时担任“膜科学与技术”期刊编委，膜学会理事（筹），膜工业协会工程与应用专业委员会及特种分离膜专业委员会委员、中国兵工学会活性炭测试分析与应用研究分会委员等。
性别：男
毕业院校：大连工学院
学位：硕士
所在单位：化工学院
学科：化学工艺. 膜科学与技术. 功能材料化学与化工
办公地点：化工综合楼A201
联系方式：微信/电话 13500711370
电子邮箱：wangth@dlut.edu.cn
Process Intensification of the Hydrogen Production Reaction Using a Carbon Membrane Reactor: Kinetics Analysis
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论文类型：期刊论文
发表时间：2017-11-01
发表刊物：ENERGY TECHNOLOGY
收录刊物：SCIE、EI、Scopus
卷号：5
期号：11
页面范围：1990-1997
ISSN号：2194-4288
关键字：carbon; copper; hydrogen production; membranes; methanol reforming
摘要：Plate carbon membranes were fabricated and coupled into a membrane reactor to intensify the steam reforming of methanol (SRM). The homemade Cu-based catalyst and carbon membranes were characterized by using thermogravimetric analysis, X-ray diffraction, N-2 adsorption, and gas permeation. The effects of the reaction temperature, reactor type, and carbon membranes on the methanol conversion and hydrogen yield were investigated. The results show that the coupling of carbon membranes in the reactor improves the methanol conversion significantly. In addition, both the methanol conversion and reaction rate increase, and the hydrogen yield first decreases then increases as the reaction temperature was elevated from 220 to 300 degrees C. This indicates that both thermodynamic and kinetic factors contribute to the intensification of SRM in the carbon membrane reactor.