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Modeling of the production of OH and O radicals in a positive pulsed corona discharge plasma

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Indexed by:期刊论文

Date of Publication:2008-09-04

Journal:6th International Symposium on Applied Plasma Science

Included Journals:SCIE、EI、CPCI-S、Scopus

Volume:83

Issue:1,SI

Page Number:238-243

ISSN No.:0042-207X

Key Words:Numerical simulation; Pulsed corona discharge; Radicals

Abstract:A mathematical model was applied to describe the behavior of OH and O radicals in positive pulsed corona discharge of N-2-H2O mixture gas. The model takes into account the generation and disappearance of radials in a pulsed corona discharge reactor by a single pulse or continuous pulses. Their concentrations were derived by considering direct electron effect on the dissociation of gaseous molecules (O-2, N-2, H2O) and subsequent excitation transfer reaction of excited oxygen atoms to produce OH radicals. The equations promoted could be solved numerically with the FORTRAN subroutine Treanor. So as to establish the validity of the model simulation, the calculated results were compared with the experimental data. Although there is some discrepancy between the calculation and experiment, the total trend is coincident. (c) 2008 Published by Elsevier Ltd.

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