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Organic Dye-Sensitized Tandem Photoelectrochemical Cell for Light Driven Total Water Splitting

Release Time:2019-03-09  Hits:

Indexed by: Journal Papers

Date of Publication: 2015-07-22

Journal: JOURNAL OF THE AMERICAN CHEMICAL SOCIETY

Included Journals: Scopus、SCIE、ESI高被引论文、EI

Volume: 137

Issue: 28

Page Number: 9153-9159

ISSN: 0002-7863

Abstract: Light driven water splitting was achieved by a tandem dye-sensitized photoelectrochemical cell with two photoactive electrodes. The photoanode is constituted by an organic dye L0 as photosensitizer and a molecular complex Ru1 as water oxidation catalyst on meso-porous TiO2, while the photocathode is constructed with an organic dye P1 as photoabsorber and a molecular complex Col as hydrogen generation catalyst on nanostructured NiO. By combining the photocathode and the photoanode, this tandem DS-PEC cell can split water by visible light under neutral pH conditions without applying any bias.

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