Release Time:2019-03-09 Hits:
Indexed by: Journal Papers
Date of Publication: 2015-07-22
Journal: JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Included Journals: Scopus、SCIE、ESI高被引论文、EI
Volume: 137
Issue: 28
Page Number: 9153-9159
ISSN: 0002-7863
Abstract: Light driven water splitting was achieved by a tandem dye-sensitized photoelectrochemical cell with two photoactive electrodes. The photoanode is constituted by an organic dye L0 as photosensitizer and a molecular complex Ru1 as water oxidation catalyst on meso-porous TiO2, while the photocathode is constructed with an organic dye P1 as photoabsorber and a molecular complex Col as hydrogen generation catalyst on nanostructured NiO. By combining the photocathode and the photoanode, this tandem DS-PEC cell can split water by visible light under neutral pH conditions without applying any bias.