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High-Performance Photoelectrochemical Cells Based on a Binuclear Ruthenium Catalyst for Visible-Light-Driven Water Oxidation

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Indexed by:期刊论文

Date of Publication:2014-10-01

Journal:CHEMSUSCHEM

Included Journals:SCIE、EI、PubMed、Scopus

Volume:7

Issue:10

Page Number:2801-2804

ISSN No.:1864-5631

Key Words:dinuclear catalysts; molecular devices; photocatalysis; ruthenium; water splitting

Abstract:Two photoanodes based on a binuclear (2) and a mononuclear ruthenium (3) water oxidation catalysts were assembled in combination with a molecular photosensitizer (1) by using a co-adsorption method. The anodes were used in dye-sensitized photoelectrochemical cells (DS-PECs) for visible-light-driven water splitting. A DS-PEC device using TiO2(1+2) as working electrode (WE) exhibits better performance than TiO2(1+3) as WE in light-driven water splitting. Detailed photoelectrochemical studies on these DS-PEC devices are discussed.

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