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论文类型：期刊论文

发表时间：2016-04-01

发表刊物：IEEE TRANSACTIONS ON PLASMA SCIENCE

收录刊物：SCIE、EI、Scopus

卷号：44

期号：4

页面范围：657-664

ISSN号：0093-3813

关键字：Electrical parameters optimization; nonthermal plasma (NTP); reactor structure optimization; volatile organic compounds (VOCs)

摘要：The effects of reactor structure parameters (wire diameter of the coil electrode, screw pitch of the coil electrode, inner diameter of the quartz tube, and packing material) and electrical parameters (power supply mode, pulse repetitive frequency, and pulse-forming capacitance) on discharge characteristics and benzene degradation have been systematically investigated in a surface/packed-bed hybrid discharge (SPBHD) reactor. The experimental results indicate that the coil electrode with a wire diameter of 1 mm and a screw pitch of 7.5 mm appears to be more advantageous with respect to both degradation efficiency and energy yield (EY). The quartz tube with larger diameter is more beneficial to benzene degradation but not for EY. The reactor packed with BaTiO3 hollow cylinders can decompose benzene more effectively than that packed with the other materials, but goes against EY. The reactor driven by bipolar pulsed power supply favors the generation of energetic electrons and active species than ac power supply, and thus accelerates benzene degradation. Increasing the pulse voltage and pulse repetitive frequency are found to be favorable for improving energy injected into the SPBHD reactor as well as the benzene degradation, while more energy is consumed. In this system, f = 50 Hz and C-p = 2 nF are the optimal pulse repetitive frequency and pulse-forming capacitance for the bipolar pulsed power, respectively, after considering the benzene degradation and EY comprehensively.