The influence of carrier envelope phase of single-cycle THz pulse on field-free orientation of NaI molecules

Release Time:2019-03-13  Hits:

Indexed by: Journal Article

Date of Publication: 2016-04-19

Journal: EUROPEAN PHYSICAL JOURNAL D

Included Journals: Scopus、SCIE

Volume: 70

Issue: 4

ISSN: 1434-6060

Abstract: The influence of the carrier envelope phase (CEP) on the field-free orientation of the NaI molecule is investigated theoretically. The molecular orientation steered by a single-cycle terahertz (THz) pulse is studied by solving exactly the time-dependent Schrodinger equation including the rovibrational degrees of freedom. We find that the field-free orientation is dependent on the central frequency and CEP of the single-cycle pulse. The CEP of single-cycle THz pulse affects the field-free orientation mainly via changing the population distributions of rotational states. By choosing the CEP of single-cycle THz pulse at the appropriate central frequency, the maximum value of the degree of field-free orientation, < cos theta >, can reach 0.80. Moreover, we find that the duration of effective orientation (vertical bar < cos theta >vertical bar >= 0.5) is relatively long in certain regions of the laser central frequency and the CEP.

Prev One:Isotope Effects on Two-Photon Population Transfer Processes of HF and DF

Next One:The influence of carrier envelope phase of single-cycle THz pulse on filed-free orientation of NaI molecule