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Highly efficient molecular nickel catalysts for electrochemical hydrogen production from neutral water

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Indexed by:期刊论文

Date of Publication:2014-11-25

Journal:CHEMICAL COMMUNICATIONS

Included Journals:SCIE、PubMed、Scopus

Volume:50

Issue:91

Page Number:14153-14156

ISSN No.:1359-7345

Abstract:A series of nickel complexes containing N-5-pentadentate ligands with different amine-to-pyridine ratios were studied for electrochemical H-2 production in neutral water and the one with a diamine-tripyridine ligand displays a TON of up to 308000 over 60 h electrolysis at -1.25 V vs. SHE, with a Faradaic efficiency of similar to 91%.

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