侯军刚

Professor   Supervisor of Doctorate Candidates   Supervisor of Master's Candidates

Gender:Male

Alma Mater:天津大学

Degree:Doctoral Degree

School/Department:化工学院

Discipline:Fine Chemicals. Applied Chemistry

Business Address:大连理工大学西部校区精细化工楼

Contact Information:jhou@dlut.edu.cn


Paper Publications

Graphene Dots Embedded Phosphide Nanosheet-Assembled Tubular Arrays for Efficient and Stable Overall Water Splitting

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Indexed by:期刊论文

Date of Publication:2017-07-26

Journal:ACS APPLIED MATERIALS & INTERFACES

Included Journals:SCIE、EI、PubMed、Scopus

Volume:9

Issue:29

Page Number:24600-24607

ISSN No.:1944-8244

Key Words:graphene dots; transition bimetallic phosphide; oxygen evolution reaction; hydrogen evolution reaction; overall water splitting

Abstract:Bifunctional electrocatalysts are highly desired for overall water splitting. Herein, the design and fabrication of three-dimensional (3D) hierarchical earth-abundant transition bimetallic phosphide arrays constructed by one-dimensional tubular array that was derived from assembling two-dimensional nanosheet framework has been reported by tailoring the Co/Ni ratio and tunable morphologies, and zero-dimensional (0D) graphene dots were embedded on Co-Ni phosphide matrix to construct 0D/2D tubular array as a highly efficient electrode in the hydrogen evolution reaction (HER) and oxygen evolution reaction (OER). On the basis of advanced merits, such as the high surface-active sites, well-dispersed graphene dots, and enhanced electron transfer capacity as well as the confinement effect of the graphene dots on the nanosheets, the integrated GDs/Co0.8Ni0.2P tubular arrays as anode and cathode exhibit excellent OER and HER performance. By use of GDs/Co0.8Ni0.2 arrays in the two-electrode setup of the device, a remarkable electrocatalytic performance for full water splitting has been achieved with a high current density of 10 mA cm-2 at 1.54 V and outstanding long-term operation stability in an alkaline environment, indicating a promising system based on nonprecious-metal electrocatalysts toward potential practical devices of overall water splitting.

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