侯军刚

Professor   Supervisor of Doctorate Candidates   Supervisor of Master's Candidates

Gender:Male

Alma Mater:天津大学

Degree:Doctoral Degree

School/Department:化工学院

Discipline:Fine Chemicals. Applied Chemistry

Business Address:大连理工大学西部校区精细化工楼

Contact Information:jhou@dlut.edu.cn


Paper Publications

Inorganic Colloidal Perovskite Quantum Dots for Robust Solar CO2 Reduction

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Indexed by:期刊论文

Date of Publication:2017-07-18

Journal:CHEMISTRY-A EUROPEAN JOURNAL

Included Journals:SCIE、EI、PubMed、Scopus

Volume:23

Issue:40

Page Number:9481-9485

ISSN No.:0947-6539

Key Words:CO2 reduction; colloidal quantum dots; perovskite; photocatalysis; solar fuels

Abstract:Inorganic perovskite quantum dots as optoelectronic materials have attracted enormous attention in light-harvesting and emitting devices. However, photocatalytic conversion based on inorganic perovskite halides has not been reported. Here, we have synthesized colloidal quantum dots (QDs, 3-12 nm) of cesium lead halide perovskites (CsPbBr3) as a new type of photocatalytic material. The band gap energies and photoluminescence (PL) spectra are tunable over the visible spectral region according to quantum size effects on an atomic scale. The increased carrier lifetime revealed by time-resolved PL spectra, indicates the efficient electron-hole separation and transfer. As expected, the CsPbBr3 QDs with high selectivity of greater than 99% achieve an efficient yield of 20.9 mmolg(-1) towards solar CO2 reduction. This work has opened a new avenue for inorganic colloidal perovskite materials as efficient photocatalysts to convert CO2 into valuable fuels.

Pre One:Graphene Dots Embedded Phosphide Nanosheet-Assembled Tubular Arrays for Efficient and Stable Overall Water Splitting

Next One:Inorganic Colloidal Perovskite Quantum Dots Realizing Robust Solar CO2 Reduction.

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侯军刚,教授,博士生导师。入选国家级青年人才,辽宁省“兴辽计划”青年拔尖人才和星海杰青。致力于发展能源催化材料的可控合成与集成组装方法,建立微纳米结构、能带结构、电荷传输与催化性能之间的构效关系,实施能源催化体系在光能、电能与化学能之间的高效转换。至今在J. Am. Chem. Soc. (3篇, IF=15)、Nature Commun. (3篇, IF=16.6)、Angew. Chem. Int. Ed. (6篇, IF=16.6)、Adv. Mater. (3, IF=29.4)Energy Environ. Sci. (4篇, IF=32.5)、Science Bulletin (IF=18.9)ACS Nano (2篇, IF=17.1)Adv. Energy Mater. (8篇, IF=27.8)、Adv. Funct. Mater. (5篇, IF=19)、Nano Energy (5篇, IF=17.6)、Appl. Catal. B-Environ (8篇, IF=22.1)、ACS Catal. (IF=12.9)、Small (IF=13.3)等国际刊物上发表论文120余篇。主持国家自然科学基金项目(4项)等。担任Journal of Energy Chemistry、SmartMat、Transactions of Tianjin University、Chinese Journal of Structural Chemistry期刊青年编委及Nature Commun.J. Am. Chem. Soc.Angew. Chem. Int. Ed.、Energ. Environ. Sci.、Adv. Mater.、Adv. Energy Mater.、Adv. Funct. Mater.、ACS Nano、ACS Catal.、Small等国际期刊审稿人。


代表性论文(影响因子IF):

(1) Lei Ran, Zhuwei Li, Bei Ran, Jiaqi Cao, Yue Zhao, Teng Shao, Yurou Song, Michael K. H. Leung, Licheng Sun and Jungang Hou,* Engineering single-atom active sites on covalent organic frameworks for boosting CO2 photoreduction, Journal of the American Chemical Society, 2022, 144, 17097-17109. (IF=15)

(2) Xiaomeng Zhang, Panlong Zhai, Yanxue Zhang, Yunzhen Wu, Chen Wang, Lei Ran, Junfeng Gao, Zhuwei Li, Bo Zhang, Zhaozhong Fan, Licheng Sun, Jungang Hou,* Engineering single-atomic Ni-N4-O sites on semiconductor photoanodes for high-performance photoelectrochemical water splitting, Journal of the American Chemical Society, 2021, 143, 20657−20669. (IF=15)

(3) Lei Ran, Shi Qiu, Panlong Zhai, Zhuwei Li, Junfeng Gao, Xiaomeng Zhang, Bo Zhang, Chen Wang, Licheng Sun, Jungang Hou,* Conformal macroporous inverse opal oxynitride-based photoanode for robust photoelectrochemical water splitting, Journal of the American Chemical Society, 2021, 143, 7402-7413. (IF=15)

(4) Panlong Zhai, Chen Wang, Yuanyuan Zhao, Yanxue Zhang, Junfeng Gao, Licheng Sun, Jungang Hou,* Regulating electronic states of nitride/hydroxide to accelerate kinetics for oxygen evolution at large current density, Nature Communications, 2023, 14, 1873. (IF=16.6)

(5) Panlong Zhai, Mingyue Xia, Yunzhen Wu, Guanghui Zhang, Junfeng Gao, Bo Zhang, Shuyan Cao, Yanting Zhang, Zhuwei Li, Zhaozhong Fan, Chen Wang, Xiaomeng Zhang, Jeffrey T. Miller, Licheng Sun, Jungang Hou,* Engineering single-atomic ruthenium catalytic sites on defective nickel-iron layered double hydroxide for overall water splitting, Nature Communications, 2021, 12, 4587. (IF=16.6)

(6) Panlong Zhai, Yanxue Zhang, Yunzhen Wu, Junfeng Gao, Bo Zhang, Shuyan Cao, Yanting Zhang, Zhuwei Li, Licheng Sun, Jungang Hou,* Engineering active sites on hierarchical transition bimetal oxides/sulfides heterostructure array enabling robust overall water splitting, Nature Communications, 2020, 11, 5462. (IF=16.6)

(7) Yurou Song, Yanhan Ren, Yuye Jiao, Shaobo Shi, Lihua Gao, Huimin Xie, Junfeng Gao, Licheng Sun, Jungang Hou,* Metal-organic framework glass catalysts from melting glass-forming cobalt-based zeolitic imidazolate framework for boosting photoelectrochemical water oxidation, Angewandte Chemie International Edition, 2023, 62, e202306420. (IF=16.6) 

(8) Yurou Song, Xiaomeng Zhang, Yanxue Zhang, Panlong Zhai, Zhuwei Li, Dingfeng Jin, Jiaqi Cao, Chen Wang, Bo Zhang, Junfeng Gao, Licheng Sun, Jungang Hou,* Engineering MoOx/MXene hole transfer layers for unexpected boosting photoelectrochemical water oxidation, Angewandte Chemie International Edition, 2022, 61, e202200946. (IF=16.6) 

(9) Zhaozhong Fan, Ruichun Luo, Yanxue Zhang, Bo Zhang, Panlong Zhai, Yanting Zhang, Chen Wang, Junfeng Gao, Wu Zhou, Licheng Sun, Jungang Hou,* Oxygen-bridged indium-nickel atomic pair as dual-metal active sites enabling synergistic electrocatalytic CO2 reduction, Angewandte Chemie International Edition, 2023, 62, e202216326. (IF=16.6)

(10) Hainan Shi, Haozhi Wang, Yichen Zhou, Jiahui Li, Panlong Zhai, Xiangyang Li, G. Gurzadyan Gargik, Jungang Hou,* Hong Yang, Xinwen Guo, Atomically dispersed indium-copper dual-metal active sites promoting C-C coupling for CO2 photoreduction to ethanol, Angewandte Chemie International Edition, 2022, 61, e202208904. (IF=16.6) 

(11) Chen Wang, Panlong Zhai, Mingyue Xia, Yunzhen Wu, Bo Zhang, Zhuwei Li, Lei Ran, Junfeng Gao, Xiaomeng Zhang, Zhaozhong Fan, Licheng Sun, Jungang Hou,* Engineering lattice oxygen activation of iridium clusters stabilized on amorphous bimetal borides array for oxygen evolution reaction, Angewandte Chemie International Edition, 2021, 60, 27126–27134. (IF=16.6) 

(12) Jungang Hou,* Huijie Cheng, Osamu Takeda, Hongmin Zhu, Three-dimensional bimetal-graphene-semiconductor coaxial nanowire arrays to harness charge flow for the photochemical reduction of carbon dioxide, Angewandte Chemie International Edition, 2015, 54, 8480−8484. (IF=16.6) 

(13) Bo Zhang, Yuan Chang, Panlong Zhai, Chen Wang, Junfeng Gao, Licheng Sun and  Jungang Hou,* Enriching metal-oxygen species and phosphate modulating of active sites for robust electrocatalytical CO2 reduction, Advanced Materials, 2023, 35, 2304379. (IF=29.4) 

(14) Yunzhen Wu, Yuanyuan Zhao, Panlong Zhai, Chen Wang, Junfeng Gao, Licheng Sun, Jungang Hou,* Triggering lattice oxygen activation of single-atomic Mo sites anchored on Ni–Fe oxyhydroxides nanoarrays for electrochemical water oxidation, Advanced Materials, 2022, 34, 2202523. (IF=29.4) 

(15) Chen Wang, Panlong Zhai, Mingyue Xia, Wei Liu, Junfeng Gao, Licheng Sun and Jungang Hou,* Identification of the origin for reconstructed active sites on oxyhydroxide for oxygen evolution reaction, Advanced Materials, 2023, 35, 2209307. (IF=29.4)

(16) Sufeng An, Guanghui Zhang, Keyan Li, Zhennan Huang, Xiang Wang, Yongkang Guo, Jungang Hou,* Chunshan Song, Xinwen Guo, Self-supporting 3D carbon nitride with tunable n→π* electronic transition for enhanced solar hydrogen production, Advanced Materials, 2021, 33, 2104361. (IF=29.4) 

(17) Yanting Zhang, Lei Ran, Yanxue Zhang, Panlong Zhai, Yunzhen Wu, Junfeng Gao, Zhuwei Li, Bo Zhang, Chen Wang, Zhaozhong Fan, Xiaomeng Zhang, Jiaqi Cao, Dingfeng Jin, Licheng Sun, Jungang Hou,* Two-dimensional defective boron-doped niobic acid nanosheets for robust nitrogen photofixation, ACS Nano, 2021, 15, 17820−17830. (IF=17.1) 

(18) Huimin Xie, Yurou Song, Yuye Jiao, Lihua Gao, Shaobo Shi, Chen Wang and Jungang Hou,* Engineering surface passivation and hole transport layer on hematite photoanodes enabling robust photoelectrocatalytic water oxidation, ACS Nano, 2024, 18, 5712-5722. (IF=17.1) 

(19) Zhuwei Li, Xiaoran Shi, Huijie Cheng, Yurou Song, Yuye Jiao, Shaobo Shi, Junfeng Gao and Jungang Hou,* Atomically dispersed iron active sites on covalent organic frameworks for artificial photosynthesis of hydrogen peroxide, Advanced Energy Materials, 2024, 14, 2302797. (IF=27.8)

(20) Yurou Song, Yunzhen Wu, Shuyan Cao, Yanxue Zhang, Degen Luo, Junfeng Gao, Zhuwei Li, Licheng Sun, Jungang Hou,* Simultaneous photoelectrocatalytic oxidation and nitrite–ammonia conversion with artificial photoelectrochemistry cells,  Advanced Energy Materials, 2022, 12, 2201782. (IF=27.8)

(21) Bo Zhang, Yuan Chang, Yunzhen Wu, Zhaozhong Fan, Panlong Zhai, Chen Wang, Junfeng Gao, Licheng Sun, Jungang Hou,* Regulating OCHO intermediate as rate-determining step of defective oxynitride nanosheets enabling robust CO2 electroreduction, Advanced Energy Materials, 2022, 12, 2200321. (IF=27.8)

(22) Yunzhen Wu, Panlong Zhai, Shuyan Cao, Zhuwei Li, Bo Zhang, Yanting Zhang, Xiaowa Nie, Licheng Sun, Jungang Hou,* Beyond d orbits: steering the selectivity of electrochemical CO2 reduction via hybridized sp band of sulfur-incorporated porous Cd architectures with dual collaborative sites, Advanced Energy Materials, 2020, 10, 2002499. (IF=27.8)

(23) Yunzhen Wu, Shuyan Cao, Jungang Hou,* Zhuwei Li, Bo Zhang, Panlong Zhai, Yanting Zhang, Licheng Sun, Rational design of nanocatalysts with nonmetal species modification for electrochemical CO2 reduction, Advanced Energy Materials, 2020, 10, 2000588. (IF=27.8)

(24) Shuyan Cao, Yunzhen Wu, Jungang Hou,* Bo Zhang, Zhuwei Li, Xiaowa Nie, Licheng Sun, 3D porous pyramid heterostructure array realizing efficient photo-electrochemical performance, Advanced Energy Materials, 2020, 10, 1902935. (IF=27.8)

(25) Bo Zhang, Jungang Hou,* Yunzhen Wu, Shuyan Cao, Zhuwei Li, Xiaowa Nie, Zhanming Gao, and Licheng Sun, Tailoring active sites in mesoporous defect-rich NC/Vo-WON heterostructure array for superior electrocatalytic hydrogen evolution, Advanced Energy Materials, 2019, 9, 1803693. (IF=27.8)

(26) Jungang Hou,* Shuyan Cao, Yunzhen Wu, Fei Liang, Yiqing Sun, Zheshuai Lin, and Licheng Sun, Atomically thin mesoporous In2O3-x/In2S3 lateral heterostructures enabling robust broadband-light photoelectrochemical water splitting, Advanced Energy Materials, 2018, 8, 1701114. (IF=27.8)

(27) Jungang Hou,* Yunzhen Wu, Shuyan Cao, Fei Liang, Zheshuai Lin, Zhanming Gao, Licheng Sun, In situ phase-induced spatial charge separation in core-shell oxynitride nanocube heterojunctions realizing robust solar water splitting, Advanced Energy Materials, 2017, 7, 1700171. (IF=27.8)

(28) Jungang Hou, Huijie Cheng, Osamu Takeda, Hongmin Zhu, Unique 3D heterojunction photoanode design to harness charge transfer for efficient and stable photoelectrochemical water splitting, Energy&Environmental Science, 2015, 8, 1348−1357. (IF=32.5)

(29) Jungang Hou, Chao Yang, Huijie Cheng, Shuqiang Jiao, Osamu Takeda and Hongmin Zhu, High-performance p-Cu2O/n-TaON heterojunction nanorod photoanodes passivated with an ultrathin carbon sheath for photoelectrochemical water splitting, Energy&Environmental Science, 2014, 7, 3758−3768. (IF=32.5)

(30) Jungang Hou, Zheng Wang, Chao Yang, Huijie Cheng, Shuqiang Jiao, Hongmin Zhu. Cobalt-bilayer catalyst decorated Ta3N5 nanorod arrays as integrated electrodes for photoelectrochemical water oxidation, Energy&Environmental Science, 2013, 6, 3322−3330. (IF=32.5)

(31) Zheng Wang, Jungang Hou, Chao Yang, Shuqiang Jiao, Kai Huang, Hongmin Zhu, Hierarchical metastable γ-TaON hollow structures for efficient visible-light water splitting, Energy&Environmental Science, 2013, 6, 2134−2144. (IF=32.5)

(32) Zhuwei Li, Shi Qiu, Yurou Song, Shiyu Huang, Junfeng Gao, Licheng Sun, Jungang Hou,* Engineering single–atom active sites anchored covalent organic frameworks for efficient metallaphotoredox C–N cross–coupling reactions, Science Bulletin, 2022, 67, 1971-1981. (IF=18.9)

(33) Shiyu Huang, Yuan Chang, Zhuwei Li, Jiaqi Cao, Yurou Song, Junfeng Gao, Licheng Sun, Jungang Hou,* Single-atom metal sites anchored hydrogen-bonded organic frameworks for superior “two-in-one” photocatalytic reaction, Advanced Functional Materials, 2023, 2211631.

(34) Jungang Hou,* Yunzhen Wu, Bo Zhang, Shuyan Cao, Zhuwei Li, and Licheng Sun, Rational design of nanoarray architectures for electrocatalytic water splitting, Advanced Functional Materials, 2019, 29, 1808367. (IF=19)

(35) Jungang Hou,* Yiqing Sun, Yunzhen Wu, Shuyan Cao, Licheng Sun, Promoting active sites in core-shell nanowire array as Mott-Schottky electrocatalysts for efficient and stable overall water splitting, Advanced Functional Materials, 2018, 28, 1704447. (IF=19)

(36) Jungang Hou,* Yiqing Sun, Zhuwei Li, Bo Zhang, Shuyan Cao, Yunzhen Wu, Zhanming Gao, Licheng Sun, Electrical behavior and electron transfer modulation of nickel-copper nanoalloys confined in nickel-copper nitrides nanowires array encapsulated in nitrogen-doped carbon framework as robust bifunctional electrocatalyst for overall water splitting, Advanced Functional Materials, 2018, 28, 1803278. (IF=19)

(37) Yunzhen Wu, Yanan Meng, Jungang Hou,* Shuyan Cao, Zhijian Wu, Licheng Sun, Orienting active crystal planes of new class lacunaris Fe2PO5 polyhedrons for robust water oxidation in alkaline and neutral media, Advanced Functional Materials, 2018, 28, 1801397. (IF=19)

(38) Jungang Hou,* Bo Zhang, Zhuwei Li, Shuyan Cao, Yiqing Sun, Yunzhen Wu, Zhanming Gao, Licheng Sun, Vertically aligned oxygenated-CoS2-MoS2 heteronanosheet architecture from polyoxometalate for efficient and stable overall water splitting, ACS Catalysis, 2018, 8, 4612−4621. (IF=12.9) 

(39) Zhuwei Li, Jungang Hou,∗ Bo Zhang, Shuyan Cao, Yunzhen Wu, Zhanming Gao, Xiaowa Nie, Licheng Sun, Two-dimensional Janus heterostructures for superior Z-scheme photocatalytic water splitting, Nano Energy, 2019, 59, 537. (IF=17.6)

(40) Jungang Hou,* Shuyan Cao, Yunzhen Wu, Fei Liang, Yongfu Sun, Zheshuai Lin, Licheng Sun, Simultaneously efficient light absorption and charge transport of phosphate and oxygen-vacancy confined in bismuth tungstate atomic layers triggering robust solar CO2 reduction, Nano Energy, 2017, 32, 359−366. (IF=17.6)

(41) Jungang Hou,* Shuyan Cao, Yunzhen Wu, Fei Liang, Lu Ye, Zheshuai Lin, Licheng Sun, Perovskite-based nanocubes with simultaneously improved visible-light absorption and charge separation enabling efficient photocatalytic CO2 reduction, Nano Energy, 2016, 30, 59−68. (IF=17.6)

(42) Kemeng Ji, Hamidreza Arandiyan, Pan Liu, Ling Zhang, Jiuhui Han, Yacong Xue, Jungang Hou,* Hongxing Dai, Interfacial insights into 3D plasmonic multijunction nanoarchitecture toward efficient photocatalytic performance, Nano Energy, 2016, 27, 515–525. (IF=17.6)

(43) Jungang Hou,* Huijie Cheng, Osamu Takeda, Hongmin Zhu, Hierarchical carbon quantum dots/hydrogenated-γ-TaON heterojunctions for broad spectrum photocatalytic performance, Nano Energy, 2015, 18, 143−153. (IF=17.6)

(44) Jungang Hou,* Yunzhen Wu, Shuyan Cao, Yiqing Sun, Licheng Sun, Active sites intercalated ultrathin carbon sheath on nanowire arrays as integrated core-shell architecture: Highly efficient and durable electrocatalysts for overall water splitting, Small 2017, 13, 1702018. (IF=13.3)

(45) Zhuwei Li, Yaning Li, Huijie Cheng, Yurou Song, Yuye Jiao, Shaobo Shi, Junfeng Gao, Licheng Sun, Jungang Hou, Atomically dispersed Ni active sites on covalent organic frameworks for heterogeneous metallaphotocatalytic C-N cross-coupling, Applied CatalysiS B-Environment and Energy, 2024, 345, 123698. (IF=22.1)

(46) Hainan Shi, Jiahui Li, Haozhi Wang, Jungang Hou,* Keyan Li, Xinwen Guo, Chlorine tailored p-d blocks dual-metal atomic catalyst for efficient photocatalytic CO2 reduction, Applied Catalysis B: Environmental, 2023, 322, 122139. (IF=22.1)

(47) Sufeng An, Yongkang Guo, Xiaoyu He, Pan Gao, Guangjin Hou, Jungang Hou,* Chunshan Song, Xinwen Guo, Intermediate-induced repolymerization for constructing self-assembly architecture: Red crystalline carbon nitride nanosheets for notable hydrogen evolution, Applied Catalysis B: Environmental, 2022, 310, 121323. (IF=22.1)

(48) Hainan Shi, Saran Long, Shen Hu, Jungang Hou,* Wenjun Ni, Chunshan Song, Keyan Li, Gagik G. Gurzadyan, Xinwen Guo, Interfacial charge transfer in 0D/2D defect-rich heterostructures for efficient solar-driven CO2 reduction, Applied Catalysis B: Environmental, 2019, 245, 760–769. (IF=22.1)

(49) Jungang Hou, Chao Yang, Zheng Wang, Shuqiang Jiao, Hongmin Zhu, Bi2O3 quantum dots decorated anatase TiO2 nanocrystals with exposed {001} facets on graphene sheets for enhanced visible-light photocatalytic performance, Applied Catalysis B: Environmental, 2013, 129, 333−341. (IF=22.1)

(50) Jungang Hou, Chao Yang, Zheng Wang, Weilin Zhou, Shuqiang Jiao, Hongmin Zhu, In-situ synthesis of α-β phase heterojunction on Bi2O3 nanowires with exceptional visible-light photocatalytic performance, Applied Catalysis B: Environmental, 2013, 142−143, 504−511. (IF=22.1)

(51) Jungang Hou, Chao Yang, Zheng Wang, Qinghuan Ji, Yitong Li, Guochao Huang, Shuqiang Jiao, Hongmin Zhu, Three-dimensional Z-scheme AgCl/Ag/γ-TaON heterostructural hollow spheres for enhanced visible-light photocatalytic performance, Applied Catalysis B: Environmental, 2013, 142−143, 579−589. (IF=22.1)

(52) Jungang Hou, Rui Cao, Shuqiang Jiao, Hongmin Zhu, R. V. Kumar, PANI/Bi12TiO20 complex architectures: Controllable synthesis and efficient visible light-driven photocatalytic activities, Applied Catalysis B: Environmental, 2011, 101, 399−406. (IF=22.1)


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